Search results for " mixed oxides"

showing 10 items of 15 documents

Reaction products and pathways in the selective oxidation of C-2-C-4 alkanes on MoVTeNb mixed oxide catalysts

2010

[EN] The catalytic properties of MoVTeNbO catalysts during the selective oxidation of short chain alkanes and olefins (C-2-C-4) have been comparatively studied The main reaction products have been ethylene from ethane acrylic acid from propane maim anhydride from n-butane and methacrolein from isobutane FTIR studies of the adsorption of the main reaction products i e olefins and aldehydes over MoVTeNbO catalyst has been carried out Accordingly the reaction pathway is explained on the basis of the characteristics of the alkane fed the stability and reactivity of both the intermediates and the reaction products and the nature of the catalytic sites involved in each reaction (C) 2010 Elsevier …

Alkanechemistry.chemical_classificationMaleic anhydrideButaneMethacroleinGeneral ChemistryAldehydeCatalysisCatalysisMoVTeNb mixed oxideschemistry.chemical_compoundchemistryIsobutaneOrganic chemistryReactivity (chemistry)Selective oxidation of alkanesIn situ FTIR spectra
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Influence of gel composition in the synthesis of MoVTeNb catalysts over their catalytic performance in partial propane and propylene oxidation

2010

[EN] MoVTeNb mixed oxides catalysts have been prepared by a slurry method with different molar compositions (Mo/Te ratio from 2 to 6 and Nb/(V + Nb) ratio from 0 to 0.7) in the synthesis gel leading to different crystalline phases distribution and catalytic behaviour in the partial oxidation of both propane and propylene to acrylic acid. Chemical analysis indicates that the composition of samples before and after the heat-treatment changes, especially the Te-content, since a significant amount of Te is lost during the heat-treatment step when the amount of oxalate (from niobium oxalate) increases in the synthesis gel. Thus, the nature of the crystalline phases and the catalytic performance …

ChemistryStereochemistryOxalic acidAcroleinGeneral ChemistryCatalysisOxalateCatalysisPropeneAcrylic acidMo–V–Te–Nb–O mixed oxideschemistry.chemical_compoundLoss of telluriumChemical engineeringPropaneOxalic acidPartial oxidationSelective propane oxidationAcrylic acid
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The Influence of Composition in Determining the Solid State Properties of Al Mixed Oxides

2011

Composition Solid State Properties Al Mixed OxidesSettore ING-IND/23 - Chimica Fisica Applicata
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Electrochemical Fabrication of High K Niobium-Tantalum Mixed Oxides/Poly 3-4 Ethylene Dioxythiophene Junctions.

2012

Electrochemical Fabrication High K Niobium-Tantalum Mixed Oxides Poly 3-4 Ethylene DioxythiopheneSettore ING-IND/23 - Chimica Fisica Applicata
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Electrochemical fabrication of high k Al-Ta mixed oxides

2014

Electrochemical fabrication high k Al-Ta mixed oxides Photoelectrochemistry Electrochemical Impedance Spectroscopy Tuning of solid state propertiesSettore ING-IND/23 - Chimica Fisica Applicata
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Heterogeneous catalytic degradation of phenolic substrates: catalysts activity

2009

This review article explored the catalytic degradation of phenol and some phenols derivates by means of advanced oxidation processes (AOPs). Among them, only the heterogeneous catalyzed processes based on catalytic wet peroxide oxidation. catalytic ozonation and catalytic wet oxidation were reviewed. Also selected recent examples about heterogeneous photocatalytic AOPs; will be presented. In details, the present review contains: (i) data concerning catalytic wet peroxide oxidation of phenolic compounds over metal-exchanged zeolites, hydrotalcites, metal-exchanged clays and resins. (ii) Use of cobalt-based catalysts, hydrotalcite-like compounds, active carbons in the catalytic ozonation proc…

Environmental EngineeringHealth Toxicology and MutagenesisHeterogeneous catalysisPeroxideCatalysisCatalysischemistry.chemical_compoundOzoneTransition metalCatalytic wet peroxide oxidation; Catalytic ozonation; Hydrotalcite-like compoundsPhenolsCatalytic wet peroxide oxidationEnvironmental ChemistryOrganic chemistryHydrotalcite-like compoundsWet oxidationZeoliteWaste Management and DisposalAcetic AcidAOPs Catalytic wet peroxide oxidation Catalytic ozonation Catalytic wet oxidation Phenol Acetic acid Metal-exchanged zeolites Hydrotalcite-like compounds Metal-exchanged/clays and resins Activated carbon Mixed oxides Noble metals CoOx/Al2O3-BaO catalystsPollutionNanomaterial-based catalystPeroxidesCatalytic oxidationchemistryMetalsCatalytic ozonationOxidation-Reduction
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Dielectric Properties of Al-Nb Amorphous Mixed Oxides

2013

Submitted by Paula Candeias (paula.candeias@lneg.pt) on 2014-02-25T11:53:22Z No. of bitstreams: 1 ECSJournalSolidStateScienceTechnology_N205.pdf: 205716 bytes, checksum: 7b6ac8703b59f9bc280a9cb4082ee0f2 (MD5) Approved for entry into archive by Paula Candeias (paula.candeias@lneg.pt) on 2014-02-25T11:53:42Z (GMT) No. of bitstreams: 1 ECSJournalSolidStateScienceTechnology_N205.pdf: 205716 bytes, checksum: 7b6ac8703b59f9bc280a9cb4082ee0f2 (MD5) Approved for entry into archive by Paula Candeias (paula.candeias@lneg.pt) on 2014-02-25T11:54:01Z (GMT) No. of bitstreams: 1 ECSJournalSolidStateScienceTechnology_N205.pdf: 205716 bytes, checksum: 7b6ac8703b59f9bc280a9cb4082ee0f2 (MD5) Made available i…

Materials scienceInorganic chemistryDielectric Propertieschemistry.chemical_elementDielectricElectronic Optical and Magnetic MaterialsAmorphous solidSettore ING-IND/23 - Chimica Fisica ApplicataMixed OxideschemistryChemical engineeringAluminiumAluminiumDielectric Properties Al-Nb amorphous mixed oxidesECS Journal of Solid State Science and Technology
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Selective propane oxidation over MoVSbO catalysts. On the preparation, characterization and catalytic behavior of M1 phase

2009

Nb-free (SbO)(2)M(20)O(56) catalysts (M = Mo, V) presenting pure M1 phase have been prepared by a post-synthesis treatment with hydrogen peroxide of a heat-treated MoVSbO mixed metal oxide catalyst previously prepared by hydrothermal method. The characterization of catalysts and their results for propane oxidation suggest that the optimization in the preparation of the M1 phase depends strongly on the washing procedure. The optimal removing of Sb species formed during post-synthesis treatment can explain the improvement in the catalytic activity; while the better selectivity to acrylic acid of the catalysts obtained by post-synthesis treatment can be explained by the elimination of M2 phase…

Post-synthesis treatmentInorganic chemistryOxideHeterogeneous catalysisCatalysisCatalysischemistry.chemical_compoundchemistryPropanePhase (matter)Hydrothermal synthesisHydrothermal synthesisPhysical and Theoretical ChemistryM1 phaseSelectivityHydrogen peroxidePropane oxidationMo–V–Sb mixed oxides
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The Effect of Anodizing Bath Composition on the Electronic Properties of Anodic Ta-Nb Mixed Oxides

2022

Anodic oxides were grown to 50 V on Ta-Nb sputtering deposited alloys, with high Nb content, in acetate ions containing an aqueous solution to study the effect of the anodizing bath composition on anodic layers’ dielectric properties. Photoelectrochemical measurements proved the presence of a photocurrent in the band gap of photon energy lower than oxides, due to optical transitions involving localized electronic states as a consequence of acetate ions incorporation. Flat band potential value estimates assessed the insulating nature of the anodic oxides grown in the acetate buffer solution. Differential capacitance measurements showed that the highest capacitance value was measured for the …

Settore ING-IND/23 - Chimica Fisica ApplicataNb oxide Ta oxide anodizing capacitance electrolytic capacitors mixed oxidesGeneral Chemical Engineeringanodizing; capacitance; electrolytic capacitors; mixed oxides; Ta oxide; Nb oxideGeneral Materials ScienceNanomaterials; Volume 12; Issue 24; Pages: 4439
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Photoelectrochemical Polymerization of 3-4 Ethylene dioxythiophene on Anodic Niobium- Tantalum Mixed Oxides.

2012

Settore ING-IND/23 - Chimica Fisica ApplicataPhotoelectrochemical Polymerization 3-4 Ethylene dioxythiophene Anodic Niobium- Tantalum Mixed Oxides
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